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Alpha decay in isotopes of atomic number less than 83

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Some time ago we started work in an attempt to observe alpha-particle decay in isotopes of atomic number less than 83. In the first experiments, thin targets of gold leaf were bombarded with 190-Me...

Some time ago we started work in an attempt to observe alpha-particle decay in isotopes of atomic number less than 83. In the first experiments, thin targets of gold leaf were bombarded with 190-Mev deuterons in the 184-inch cyclotron. Two alpha-decay periods were observed in these targets; one of 0.7 minutes half-life and another of 4.3 minutes half-life. The alpha-particle energies were 5.7 and 5.2 Mev, respectively. Chemical separations proved that the 4.3-minute period is due to a gold isotope and suggested that the 0.7-minute period is due to a mercury isotope. The mass numbers of these new isotopes have not been determined. However, the results of excitation-functions in the production of the gold isotope by bombarding gold and platinum with protons suggest that its mass number lies in the range 185-188. The work on this isotope indicates that the alpha to electron capture branching ratio is of the order of magnitude of 10⁻⁴, and that positron activity accompanies the 4.3-minute alpha-period.

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